Mobility and persistence of methane in groundwater in a controlled-release field experiment

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dc.contributor.authorCahill, Aaron G.
dc.contributor.authorSteelman, Colby M.
dc.contributor.authorForde, Olenka
dc.contributor.authorKuloyo, Olukayode
dc.contributor.authorEmil Ruff, S.
dc.contributor.authorMayer, Bernhard
dc.contributor.authorUlrich Mayer, K.
dc.contributor.authorStrous, Marc
dc.contributor.authorCathryn Ryan, M.
dc.contributor.authorCherry, John A.
dc.contributor.authorParker, Beth L.
dc.date.accessioned2023-03-01T22:14:46Z
dc.date.available2023-03-01T22:14:46Z
dc.date.issued2017-04
dc.description.abstractExpansion of shale gas extraction has fuelled global concern about the potential impact of fugitive methane on groundwater and climate. Although methane leakage from wells is well documented, the consequences on groundwater remain sparsely studied and are thought by some to be minor. Here we present the results of a 72-day methane gas injection experiment into a shallow, flat-lying sand aquifer. In our experiment, although a significant fraction of methane vented to the atmosphere, an equal portion remained in the groundwater. We find that methane migration in the aquifer was governed by subtle grain-scale bedding that impeded buoyant free-phase gas flow and led to episodic releases of free-phase gas. The result was lateral migration of gas beyond that expected by groundwater advection alone. Methane persisted in the groundwater zone despite active growth of methanotrophic bacteria, although much of the methane that vented into the vadose zone was oxidized. Our findings demonstrate that even small-volume releases of methane gas can cause extensive and persistent free phase and solute plumes emanating from leaks that are detectable only by contaminant hydrogeology monitoring at high resolution.en_US
dc.identifier.citationCahill, A. G., Steelman, C. M., Forde, O., Kuloyo, O., Emil Ruff, S., Mayer, B., Ulrich Mayer, K., Strous, M., Cathryn Ryan, M., Cherry, J. A., & Parker, B. L. (2017). Mobility and persistence of methane in groundwater in a controlled-release field experiment. Nature Geoscience, 10(4), Article 4. https://doi.org/10.1038/ngeo2919en_US
dc.identifier.doihttps://doi.org/10.1038/ngeo2919en_US
dc.identifier.urihttp://hdl.handle.net/1880/115891
dc.identifier.urihttps://doi.org/10.11575/PRISM/46073
dc.language.isoengen_US
dc.publisherNature Publishing Groupen_US
dc.publisher.facultyScienceen_US
dc.publisher.hasversionacceptedVersionen_US
dc.publisher.institutionUniversity of Calgaryen_US
dc.publisher.policyhttps://www.nature.com/neuro/editorial-policies/self-archiving-and-license-to-publishen_US
dc.rightsUnless otherwise indicated, this material is protected by copyright and has been made available with authorization from the copyright owner. You may use this material in any way that is permitted by the Copyright Act or through licensing that has been assigned to the document. For uses that are not allowable under copyright legislation or licensing, you are required to seek permission.en_US
dc.titleMobility and persistence of methane in groundwater in a controlled-release field experimenten_US
dc.typejournal articleen_US
ucalgary.item.requestcopyfalseen_US
ucalgary.scholar.levelFacultyen_US
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